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Page 449
order of 1 to 3 years (Hunten, 1975). It seems to be generally
accepted that volcanic aerosols remain in the stratosphere for
several years (Kellogg and Schneider, 1974; Ramaswamy and Kiehl,
1985). A screen could be created in the stratosphere by adding more
dust to the natural stratospheric dust to increase its net
reflection of sunlight.
An alternative to dust is sulfuric acid aerosol, the other
principal natural component of stratospheric haze. Dust seems a
better choice because it is similar to dust from natural soil and
so should have no noticeable effect on the ground as it gradually
falls into the troposphere and rains out. (Other possible effects
are referred to below.) However, Budyko (1982) suggests the use of
sulfuric acid aerosol, to be created by the burning of sulfur in
situ, resulting in sulfur dioxide (SO2), which will automatically absorb
atmospheric water to result in droplets of sulfuric acid solution.
He gives the required tonnage of sulfuric acid to reduce the total
radiation by 1 percent as 600,000 t. As we will see, this is less
than one-tenth of the amount we estimate is required as dust.
Budyko goes on to point out that the amount of sulfur required to
be burnt in the stratosphere to produce the aerosol is 200,000 t,
or possibly even as little as 40 percent of this, depending on the
amount of water that might be absorbed from the air. Thus the lift
requirements might be only one-seventh to one-third of that
estimated for sulfuric acid itself. He also assumes 2 years as the
lifetime of the aerosol in the stratosphere. In any case, Budyko's
maximum requirement is much less than we use below to estimate the
cost of the material and lift requirements. (Sulfur costs are about
$0.05/pound, and we assume less than $0.25/pound for dust.) The
costs to do the screening using sulfuric acid aerosol in the
stratosphere would be less than those which are estimated below for
dust, if we use the estimates of Budyko.
The amount of dust emitted into the atmosphere from natural and
manmade (mostly natural) sources is noted (from material quoted by
Toon and Pollack, 1976) to be about 1 to 3 Gt/yr, or 1 to 3 ×
1012 kg/yr.8 This is about 100 to 300 times the
amount proposed below to be added to the atmosphere.
Mass Estimates
Ramaswamy and Kiehl (1985) estimate that an aerosol dust loading
of 0.2 g/m2 for dust with a radius
of about 0.26 µm increases the planetary albedo by 12
percent, resulting in a 15 percent decrease of solar flux reaching
the surface. Since an approximately 1 percent change in solar flux
is required, and their Figures 13 and 15 suggest that, at these
loadings, the dust effects may reasonably be extrapolated downward
linearly, estimates will be made by using a dust loading of 0.02
g/m2 with a particle radius of
0.26 µm.